Relaxation Oscillations of an Exciton-Polariton Condensate Driven by Parametric Scattering.

Tian, Chuan; Chen, Linqi; Zhang, Yingjun; Zhu, Liqing; Hu, Wenping; Pan, Yichun; Wang, Zheng; Zhang, Fangxin et al. · Nano Lett · 2022

basic_science · Level V

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Abstract

We report the observation of coherent oscillations in the relaxation dynamics of an exciton-polariton condensate that were driven by parametric scattering processes. As a result of the interbranch scattering scheme and the nonlinear polariton-polariton interactions, such parametric scatterings exhibit a high scattering efficiency that leads to the fast depletion of the polariton condensate and the periodic shut-off of the bosonic stimulation processes, eventually causing relaxation oscillations. Employing polariton-reservoir interactions, the oscillation dynamics in the time domain can be projected onto the energy space. In theory, our simulations using the open-dissipative Gross-Pitaevskii equation are in excellent agreement with experimental observations. Surprisingly, the oscillation patterns, including many excitation pulses, are clearly visible in our time-integrated images, implying the high stability of the relaxation oscillations driven by polariton parametric scatterings.