Cylindrical Metalens for Generation and Focusing of Free-Electron Radiation.

Karnieli, Aviv; Roitman, Dolev; Liebtrau, Matthias; Tsesses, Shai; Van Nielen, Nika; Kaminer, Ido; Arie, Ady; Polman, Albert · Nano Lett · 2022

basic_science · Level V

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Abstract

Metasurfaces constitute a powerful approach to generate and control light by engineering optical material properties at the subwavelength scale. Recently, this concept was applied to manipulate free-electron radiation phenomena, rendering versatile light sources with unique functionalities. In this Letter, we experimentally demonstrate spectral and angular control over coherent light emission by metasurfaces that interact with free-electrons under grazing incidence. Specifically, we study metalenses based on chirped metagratings that simultaneously emit and shape Smith-Purcell radiation in the visible and near-infrared spectral regime. In good agreement with theory, we observe the far-field signatures of strongly convergent and divergent cylindrical radiation wavefronts using <i>in situ</i> hyperspectral angle-resolved light detection in a scanning electron microscope. Furthermore, we theoretically explore simultaneous control over the polarization and wavefront of Smith-Purcell radiation via a split-ring-resonator metasurface, enabling tunable operation by spatially selective mode excitation at nanometer resolution. Our work highlights the potential of merging metasurfaces with free-electron excitations for versatile and highly tunable radiation sources in wide-ranging spectral regimes.