Ultrafast Demagnetization Control in Magnetophotonic Surface Crystals.

Mishra, Kshiti; Rowan-Robinson, Richard M; Ciuciulkaite, Agne; Davies, Carl S; Dmitriev, Alexandre; Kapaklis, Vassilios; Kimel, Alexey V; Kirilyuk, Andrei · Nano Lett · 2022

basic_science · Level V

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Abstract

Magnetic memory combining plasmonics and magnetism is poised to dramatically increase the bit density and energy efficiency of light-assisted ultrafast magnetic storage, thanks to nanoplasmon-driven enhancement and confinement of light. Here we devise a new path for that, simultaneously enabling light-driven bit downscaling, reduction of the required energy for magnetic memory writing, and a subtle control over the degree of demagnetization in a magnetophotonic surface crystal. It features a regular array of truncated-nanocone-shaped Au-TbCo antennas showing both localized plasmon and surface lattice resonance modes. The ultrafast magnetization dynamics of the nanoantennas show a 3-fold resonant enhancement of the demagnetization efficiency. The degree of demagnetization is further tuned by activating surface lattice modes. This reveals a platform where ultrafast demagnetization is localized at the nanoscale and its extent can be controlled at will, rendering it multistate and potentially opening up so-far-unforeseen nanomagnetic neuromorphic-like systems operating at femtosecond time scales controlled by light.