Switching the Moiré Lattice Models in the Twisted Bilayer WSe<sub>2</sub> by Strain or Pressure.
basic_science · Level V
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- Record sourced from PubMed, PMID 37585490.
- Also identified by DOI 10.1021/acs.nanolett.3c01756.
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Abstract
Moiré superlattices of twisted van der Waals heterostructures provide a promising and tunable platform for simulating correlated two-dimensional physical models. In twisted bilayer transition-metal dichalcogenides with twist angles close to 0°, the Γ and <i>K</i> valley moiré bands are described by the honeycomb and the triangular effective lattice models, respectively, with distinct physics. Using large-scale first-principles calculations, we show that in-plane biaxial strain and out-of-plane pressure provide effective knobs for switching the moiré lattice models that emerged at the band edges in twisted bilayer WSe<sub>2</sub> by shifting the energy positions of the Γ and <i>K</i> valley minibands. The shifting mechanism originates from the differences in the orbital characters of the Γ and <i>K</i> valley states and their responses to strain and pressure. The critical strain and pressure for switching the Γ/<i>K</i> valleys are 2.11% and 2.175 GPa, respectively.