Scalable Production of 2D Material Heterostructure Textiles for High-Performance Wearable Supercapacitors.

Islam, Md Rashedul; Afroj, Shaila; Karim, Nazmul · ACS Nano · 2023

basic_science · Level V

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Abstract

Wearable electronic textiles (e-textiles) have emerged as a promising platform for seamless integration of electronic devices into everyday life, enabling nonintrusive monitoring of human health. However, the development of efficient, flexible, and scalable energy storage solutions remains a significant challenge for powering such devices. Here, we address this challenge by leveraging the distinct properties of two-dimensional (2D) material based heterostructures to enhance the performance of wearable textile supercapacitors. We report a highly scalable and controllable synthesis method for graphene and molybdenum disulfide (MoS<sub>2</sub>) through a microfluidization technique. Subsequently, we employ an ultrafast and industry-scale hierarchical deposition approach using a pad-dry method to fabricate 2D heterostructure based textiles with various configurations suitable for wearable e-textiles applications. Comparative analyses reveal the superior performance of wearable textile supercapacitors based on 2D material heterostructures, demonstrating excellent areal capacitance (∼105.08 mF cm<sup>-2</sup>), high power density (∼1604.274 μW cm<sup>-2</sup>) and energy density (∼58.377 μWh cm<sup>-2</sup>), and outstanding capacitive retention (∼100% after 1000 cycles). Our findings highlight the pivotal role of 2D material based heterostructures in addressing the challenges of performance and scalability in wearable energy storage devices, facilitating large-scale production of high-performance wearable supercapacitors.