The Wiedemann-Franz law in doped Mott insulators without quasiparticles.

Wang, Wen O; Ding, Jixun K; Schattner, Yoni; Huang, Edwin W; Moritz, Brian; Devereaux, Thomas P · Science · 2023

basic_science · Level V

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Abstract

Many metallic quantum materials display anomalous transport phenomena that defy a Fermi liquid description. Here, we use numerical methods to calculate thermal and charge transport in the doped Hubbard model and observe a crossover separating high- and low-temperature behaviors. Distinct from the behavior at high temperatures, the Lorenz number [Formula: see text] becomes weakly doping dependent and less sensitive to parameters at low temperatures. At the lowest numerically accessible temperatures, [Formula: see text] roughly approaches the Wiedemann-Franz constant [Formula: see text], even in a doped Mott insulator that lacks well-defined quasiparticles. Decomposing the energy current operator indicates a compensation between kinetic and potential contributions, which may help to clarify the interpretation of transport experiments beyond Boltzmann theory in strongly correlated metals.