Iron-sulfur chemistry can explain the ultraviolet absorber in the clouds of Venus.

Jiang, Clancy Zhijian; Rimmer, Paul B; Lozano, Gabriella G; Tosca, Nicholas J; Kufner, Corinna L; Sasselov, Dimitar D; Thompson, Samantha J · Sci Adv · 2024

basic_science · Level V

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Abstract

The clouds of Venus are believed to be composed of sulfuric acid (H<sub>2</sub>SO<sub>4</sub>) and minor constituents including iron-bearing compounds, and their respective concentrations vary with height in the thick Venusian atmosphere. This study experimentally investigates possible iron-bearing mineral phases that are stable under the unique conditions within Venusian clouds. Our results demonstrate that ferric iron can react with sulfuric acid to form two mineral phases: rhomboclase [(H<sub>5</sub>O<sub>2</sub>)Fe(SO<sub>4</sub>)<sub>2</sub>·3H<sub>2</sub>O] and acid ferric sulfate [(H<sub>3</sub>O)Fe(SO<sub>4</sub>)<sub>2</sub>]. A combination of these two mineral phases and dissolved Fe<sup>3+</sup> in varying concentrations of sulfuric acid are shown to be good candidates for explaining the 200- to 300-nm and 300- to 500-nm features of the reported unknown UV absorber. We, therefore, hypothesize a rich and largely unexplored heterogeneous chemistry in the cloud droplets of Venus that has a large effect on the optical properties of the clouds and the behavior of trace gas species throughout Venus's atmosphere.