Motion and teleportation of polar bubbles in low-dimensional ferroelectrics.

Prokhorenko, S; Nahas, Y; Govinden, V; Zhang, Q; Valanoor, N; Bellaiche, L · Nat Commun · 2024

basic_science · Level V

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Abstract

Electric bubbles are sub-10nm spherical vortices of electric dipoles that can spontaneously form in ultra-thin ferroelectrics. While the static properties of electric bubbles are well established, little to nothing is known about the dynamics of these particle-like structures. Here, we reveal pathways to realizing both the spontaneous and controlled dynamics of electric bubbles in ultra-thin Pb(Zr<sub>0.4</sub>Ti<sub>0.6</sub>)O<sub>3</sub> films. In low screening conditions, we find that electric bubbles exhibit thermally-driven chaotic motion giving rise to a liquid-like state. In the high screening regime, we show that bubbles remain static but can be continuously displaced by a local electric field. Additionally, we predict and experimentally demonstrate the possibility of bubble teleportation - a process wherein a bubble is transferred to a new location via a single electric field pulse of a PFM tip. Finally, we attribute the discovered phenomena to the hierarchical structure of the energy landscape.