Interfacial magnetic spin Hall effect in van der Waals Fe<sub>3</sub>GeTe<sub>2</sub>/MoTe<sub>2</sub> heterostructure.

Dai, Yudi; Xiong, Junlin; Ge, Yanfeng; Cheng, Bin; Wang, Lizheng; Wang, Pengfei; Liu, Zenglin; Yan, Shengnan et al. · Nat Commun · 2024

basic_science · Level V

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Abstract

The spin Hall effect (SHE) allows efficient generation of spin polarization or spin current through charge current and plays a crucial role in the development of spintronics. While SHE typically occurs in non-magnetic materials and is time-reversal even, exploring time-reversal-odd (T-odd) SHE, which couples SHE to magnetization in ferromagnetic materials, offers a new charge-spin conversion mechanism with new functionalities. Here, we report the observation of giant T-odd SHE in Fe<sub>3</sub>GeTe<sub>2</sub>/MoTe<sub>2</sub> van der Waals heterostructure, representing a previously unidentified interfacial magnetic spin Hall effect (interfacial-MSHE). Through rigorous symmetry analysis and theoretical calculations, we attribute the interfacial-MSHE to a symmetry-breaking induced spin current dipole at the vdW interface. Furthermore, we show that this linear effect can be used for implementing multiply-accumulate operations and binary convolutional neural networks with cascaded multi-terminal devices. Our findings uncover an interfacial T-odd charge-spin conversion mechanism with promising potential for energy-efficient in-memory computing.