High-performance ferroelectric field-effect transistors with ultra-thin indium tin oxide channels for flexible and transparent electronics.

Li, Qingxuan; Wang, Siwei; Li, Zhenhai; Hu, Xuemeng; Liu, Yongkai; Yu, Jiajie; Yang, Yafen; Wang, Tianyu et al. · Nat Commun · 2024

basic_science · Level V

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Abstract

With the development of wearable devices and hafnium-based ferroelectrics (FE), there is an increasing demand for high-performance flexible ferroelectric memories. However, developing ferroelectric memories that simultaneously exhibit good flexibility and significant performance has proven challenging. Here, we developed a high-performance flexible field-effect transistor (FeFET) device with a thermal budget of less than 400 °C by integrating Zr-doped HfO<sub>2</sub> (HZO) and ultra-thin indium tin oxide (ITO). The proposed FeFET has a large memory window (MW) of 2.78 V, a high current on/off ratio (I<sub>ON</sub>/I<sub>OFF</sub>) of over 10<sup>8</sup>, and high endurance up to 2×10<sup>7</sup> cycles. In addition, the FeFETs under different bending conditions exhibit excellent neuromorphic properties. The device exhibits excellent bending reliability over 5×10<sup>5</sup> pulse cycles at a bending radius of 5 mm. The efficient integration of hafnium-based ferroelectric materials with promising ultrathin channel materials (ITO) offers unique opportunities to enable high-performance back-end-of-line (BEOL) compatible wearable FeFETs for edge intelligence applications.