Self-Assembly Enabled Printable Asymmetric Self-Insulated Stretchable Conductor for Human Interface.

Ahmed, Salahuddin; Momin, Marzia; Ren, Jiashu; Lee, Hyunjin; Zhou, Tao · Adv Mater · 2024

basic_science · Level V

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Abstract

Soft and stretchable conductors with high electrical conductivity and tissue-like mechanical properties are crucial for both on-skin and implantable electronic devices. Liquid metal-based conductors hold great promise due to their metallic conductivity and minimal stiffness. However, the surface oxidation of liquid metal particles in polymeric matrices poses a challenge in forming a continuous pathway for highly conductive elastic composites. Here, it is reported a printable composite material based on liquid metal and conducting polymer that undergoes a self-assembly process, achieving high conductivity (2089 S cm<sup>-1</sup>) in the bottom surface while maintaining an insulated top surface, high stretchability (>800%), and a modulus akin to human skin tissue. This material is further applied to fabricate skin-interfaced strain sensors and electromyogram sensors through 3D printing.

Medical subject headings