Selective Excitation of Exciton-Polariton Condensate Modes in an Annular Perovskite Microcavity.

Xiong, Zhenyu; Wu, Hao; Cai, Yuanwen; Zhai, Xiaokun; Liu, Tong; Li, Baili; Song, Tieling; Guo, Longfei et al. · Nano Lett · 2024

basic_science · Level V

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Abstract

Exciton-polariton systems composed of a light-matter quasi-particle with a light effective mass easily realize Bose-Einstein condensation. In this work, we constructed an annular trap in a halide perovskite semiconductor microcavity and observed the spontaneous formation of symmetrical petal-shaped exciton-polariton condensation in the annular trap at room temperature. In our study, we found that the number of petals of the petal-shaped exciton-polariton condensates, which is decided by the orbital angular momentum, is dependent on the light intensity distribution. Therefore, the selective excitation of perovskite microcavity exciton-polariton condensates under all-optical control can be realized by adjusting the light intensity distribution. This could pave the way to room-temperature topological devices, optical cryptographical devices, and new quantum gyroscopes in the exciton-polariton system.