Correlation-driven nonequilibrium exciton site transition in a WSe<sub>2</sub>/WS<sub>2</sub> moiré supercell.

Kim, Jinjae; Park, Jiwon; Choi, Hyojin; Kim, Taeho; Cha, Soonyoung; Lee, Yewon; Watanabe, Kenji; Taniguchi, Takashi et al. · Nat Commun · 2024

basic_science · Level V

Where this comes from

Abstract

Moiré superlattices of transition metal dichalcogenides offer a unique platform to explore correlated exciton physics with optical spectroscopy. Whereas the spatially modulated potentials evoke that the exciton resonances are distinct depending on a site in a moiré supercell, there have been no clear demonstration how the moiré excitons trapped in different sites dynamically interact with the doped carriers; so far the exciton-electron dynamic interactions were presumed to be site-dependent. Thus, the transient emergence of nonequilibrium correlations are open questions, but existing studies are limited to steady-state optical measurements. Here we report experimental fingerprints of site-dependent exciton correlations under continuous-wave as well as ultrashort optical excitations. In near-zero angle-aligned WSe<sub>2</sub>/WS<sub>2</sub> heterobilayers, we observe intriguing polarization switching and strongly enhanced Pauli blocking near the Mott insulating state, dictating the dominant correlation-driven effects. When the twist angle is near 60°, no such correlations are observed, suggesting the strong dependence of atomic registry in moiré supercell configuration. Our studies open the door to largely unexplored nonequilibrium correlations of excitons in moiré superlattices.