Nonvolatile optical phase shift in ferroelectric hafnium zirconium oxide.

Taki, Kazuma; Sekine, Naoki; Watanabe, Kouhei; Miyatake, Yuto; Akazawa, Tomohiro; Sakumoto, Hiroya; Toprasertpong, Kasidit; Takagi, Shinichi et al. · Nat Commun · 2024

basic_science · Level V

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Abstract

A nonvolatile optical phase shifter is a critical component for enabling the fabrication of programmable photonic integrated circuits on a Si photonics platform, facilitating communication, computing, and sensing. Although ferroelectric materials such as BaTiO<sub>3</sub> offer nonvolatile optical phase shift capabilities, their compatibility with complementary metal-oxide-semiconductor fabs is limited. Hf<sub>0.5</sub>Zr<sub>0.5</sub>O<sub>2</sub> is an emerging ferroelectric material, which exhibits complementary metal-oxide-semiconductor compatibility. Although extensively studied for ferroelectric transistors and memories, its application to photonics remains relatively unexplored. Here, we show the optical phase shift induced by ferroelectric Hf<sub>0.5</sub>Zr<sub>0.5</sub>O<sub>2</sub>. We observed a negative change in refractive index at a 1.55 μm wavelength in a pristine device regardless of the direction of the applied electric field. The nonvolatile phase shift was only observed once in a pristine device. This non-reversible phase shift can be attributed to the spontaneous polarization within the Hf<sub>0.5</sub>Zr<sub>0.5</sub>O<sub>2</sub> film along the external electric field.