'Rewritable' and 'liquid-specific' recognizable wettability pattern.

Dhar, Manideepa; Sarkar, Debasmita; Das, Avijit; Rahaman, S K Asif; Ghosh, Dibyendu; Manna, Uttam · Nat Commun · 2024

basic_science · Level V

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Abstract

Bio-inspired surfaces with wettability patterns display a unique ability for liquid manipulations. Sacrificing anti-wetting property for confining liquids irrespective of their surface tension (γ<sub>LV</sub>), remains a widely accepted basis for developing wettability patterns. In contrast, we introduce a 'liquid-specific' wettability pattern through selectively sacrificing the slippery property against only low γ<sub>LV</sub> (<30 mN m<sup>-1</sup>) liquids. This design includes a chemically reactive crystalline network of phase-transitioning polymer, which displays an effortless sliding of both low and high γ<sub>LV</sub> liquids. Upon its strategic chemical modification, droplets of low γ<sub>LV</sub> liquids fail to slide, rather spill arbitrarily on the tilted interface. In contrast, droplets of high γ<sub>LV</sub> liquids continue to slide on the same modified interface. Interestingly, the phase-transition driven rearrangement of crystalline network allows to revert the slippery property against low γ<sub>LV</sub> liquids. Here, we report a 'rewritable' and 'liquid-specific' wettability pattern for high throughput screening, separating, and remoulding non-aqueous liquids.