Wafer-Scale Fabrication of Wearable All-Carbon Nanotube Photodetector Arrays.

Liu, Peng; Ding, Er-Xiong; Xu, Zhenyu; Cui, Xiaoqi; Du, Mingde; Zeng, Weijun; Karakassides, Anastasios; Zhang, Jin et al. · ACS Nano · 2024

basic_science · Level V

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Abstract

With electronic devices evolving toward portable and high-performance wearables, the constraints of complex and wet processing technologies become apparent. This study presents a scalable photolithography/chemical-free method for crafting wearable all-carbon nanotube (CNT) photodetector device arrays. Laser-assisted patterning and dry deposition techniques directly assemble gas-phase CNTs into flexible devices without any lithography or lift-off processes. The resulting wafer-scale all-CNT photodetector arrays showcase excellent uniformity, wearability, environmental stability, and notable broadband photoresponse, boasting a high responsivity of 44 AW<sup>-1</sup> and a simultaneous detectivity of 1.9 × 10<sup>9</sup> Jones. This research provides an efficient, versatile, and scalable strategy for manufacturing wearable all-CNT device arrays, allowing widespread adoption in wearable optoelectronics and multifunctional sensors.