Ag<sub>2</sub>Se as a tougher alternative to n-type Bi<sub>2</sub>Te<sub>3</sub> thermoelectrics.

Liu, Min; Zhang, Xinyue; Zhang, Shuxian; Pei, Yanzhong · Nat Commun · 2024

basic_science · Level V

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Abstract

For half a century, only Bi<sub>2</sub>Te<sub>3</sub>-based thermoelectrics have been commercialized for near room temperature applications including both power generation and refrigeration. Because of the strong layered structure, Bi<sub>2</sub>Te<sub>3</sub> in particular for n-type conduction has to be texturized to utilize its high in-plane thermoelectric performance, leaving a substantial challenge in toughness. This work presents the fabrication and performance evaluation of thermoelectric modules based on n-type Ag<sub>2</sub>Se paring with commercial p-Bi<sub>2</sub>Te<sub>3</sub>. Ag<sub>2</sub>Se mechanically allows an order of magnitude larger fracture strain and thermoelectrically secures the module efficiency quite competitive to that of commercial one for both refrigeration and power generation within ± 50 K of room temperature, enabling a demonstration of a significantly tougher alternative to n-type Bi<sub>2</sub>Te<sub>3</sub> for practical applications.