Crystallographic Spin Torque Conductivity Tensor of Epitaxial IrO<sub>2</sub> Thin Films for Oxide Spintronics.

Patton, Michael; Pharis, Daniel A; Gurung, Gautam; Huang, Xiaoxi; Noh, Gahee; Tsymbal, Evgeny Y; Choi, Si-Young; Ralph, Daniel C et al. · Adv Mater · 2025

basic_science · Level V

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Abstract

Unconventional spin-orbit torques arising from electric-field-generated spin currents in anisotropic materials have promising potential for spintronic applications, including for perpendicular magnetic switching in high-density memory applications. Here, all the independent elements of the spin torque conductivity tensor allowed by bulk crystal symmetries for the tetragonal conductor IrO<sub>2</sub> are determined via measurements of conventional (in-plane) anti-damping torques for IrO<sub>2</sub> thin films in the high-symmetry (001) and (100) orientations. It is then tested whether rotational transformations of this same tensor can predict both the conventional and unconventional anti-damping torques for IrO<sub>2</sub> thin films in the lower-symmetry (101), (110), and (111) orientations, finding good agreement. The results confirm that spin-orbit torques from all these orientations are consistent with the bulk symmetries of IrO<sub>2</sub>, and show how simple measurements of conventional torques from high-symmetry orientations of anisotropic thin films can provide an accurate prediction of the unconventional torques from lower-symmetry orientations.