Hyperbolic phonon-polariton electroluminescence in 2D heterostructures.

Abstract

Phonon polaritons are quasiparticles resulting from the coherent coupling of photons with optical phonons in polar dielectrics¹. Owing to their exceptional ability to confine electric fields to deep-subwavelength scales with low loss, they are uniquely poised to enable a suite of applications beyond the reach of conventional photonics, such as subdiffraction imaging² and near-field energy transfer^3-5. The conventional approach to exciting phonon polaritons through optical methods, however, involves costly light sources along with near-field schemes^6,7, and generally leads to low excitation efficiency owing to substantial momentum mismatch between phonon polaritons and free-space photons. Here we demonstrate that under proper conditions, phonon polaritons can be excited all-electrically by drifting charge carriers. Specifically, in hexagonal boron nitride (hBN)/graphene heterostructures, by electrically driving charge carriers in ultrahigh-mobility graphene out of equilibrium, we observe bright electroluminescence of hBN's hyperbolic phonon polaritons (HPhPs) at mid-infrared frequencies, which shows a temperature and carrier density dependence distinct from black-body thermal emission. Moreover, the carrier density dependence of the HPhP electroluminescence spectra reveals that HPhP electroluminescence can arise from both interband transition and intraband Cherenkov radiation⁸ of charge carriers in graphene. The HPhP electroluminescence offers avenues for realizing electrically pumped mid-infrared and terahertz phonon-polariton light sources.