Pressure-Driven One-Dimensional Superlattices in Monolayer Crystals on a Vicinal Surface.
basic_science · Level V
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- Record sourced from PubMed, PMID 40240306.
- Also identified by DOI 10.1021/acs.nanolett.4c06687.
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Abstract
A 1D superlattice can be imposed on monolayer materials by the periodic atomic steps of a vicinal crystalline surface. By means of the rotational anisotropy of second harmonic generation, we demonstrate that the periodic modulation of monolayer WS<sub>2</sub> by the diamond (230) surface gives rise to an orientation-dependent breaking of crystal symmetry, a fundamental prerequisite for generation of a one-dimensional superlattice from a two-dimensional lattice, when subjected to external pressure. These observations contrast with the case of monolayer WS<sub>2</sub> on the diamond (100) surface, which largely retains its 3-fold rotational symmetry when pressure is applied. Vicinal surfaces offer a potentially versatile approach to the nanoscale periodic in-plane modulation of layered crystals and engineering their electronic and optical functionality.