Superconducting gap of H<sub>3</sub>S measured by tunnelling spectroscopy.

Du, Feng; Drozdov, Alexander P; Minkov, Vasily S; Balakirev, Fedor F; Kong, Panpan; Smith, G Alexander; Yan, Jiafeng; Shen, Bin et al. · Nature · 2025

basic_science · Level V

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Abstract

Several hydrogen-rich superconductors have been found to show unprecedentedly high critical temperatures<sup>1-4</sup>, stimulating investigations into the nature of the superconductivity in these materials. Although their macroscopic superconducting properties are established<sup>1,5-7</sup>, microscopic insights into the pairing mechanism remains unclear. Here we characterize the superconducting gap structure in the high-temperature superconductor H<sub>3</sub>S and its deuterium counterpart D<sub>3</sub>S by performing tunnelling spectroscopy measurements. The tunnelling spectra reveal that H<sub>3</sub>S and D<sub>3</sub>S both have a fully gapped structure, which could be well described by a single s-wave Dynes model, with gap values 2Δ of approximately 60 meV and 44 meV, respectively. Furthermore, we observed gap features of another likely H-depleted H<sub>x</sub>S superconducting phase in a poorly synthesized hydrogen sulfide sample. Our work offers direct experimental evidence for superconductivity in the hydrogen-rich superconductor H<sub>3</sub>S from a microscopic perspective. It validates the phonon-mediated mechanism of superconducting pairing and provides a foundation for further understanding the origins of high-temperature superconductivity in hydrogen-rich compounds.