Far-field femtosecond laser-driven λ/73 super-resolution fabrication of 2D van der Waals NbOI<sub>2</sub> nanostructures in ambient air.
basic_science · Level V
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- Record sourced from PubMed, PMID 40320417.
- Also identified by DOI 10.1038/s41467-025-59520-9 and PMC identifier 12050275.
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Abstract
The design and fabrication of ultrafine nanostructures in two-dimensional (2D) van der Waals materials are crucial for the functionalization of electronic devices. Here, we report the utilization of far-field femtosecond laser patterning to fabricate super-resolution nano-groove array (NGA) structures in 2D multilayer NbOI<sub>2</sub> in ambient air, achieving groove widths as low as ~14.5 nm (~λ/73). The NGA structures maintain a well-defined single-crystal NbOI<sub>2</sub> with amorphous Nb<sub>2</sub>O<sub>5</sub> edges as narrow as 3.2 nm. The formation mechanism of NGA structure is confirmed to be associated with the coupled field of surface plasmon polariton periodic field and nano-groove-induced local near-field induced by femtosecond laser irradiation. Furthermore, the NGA-NbOI<sub>2</sub> gas sensor exhibits NO<sub>2</sub> sensing performance, with a rapid response time (5.1 s), which is attributed to the existence of abundant NbOI<sub>2</sub>-Nb<sub>2</sub>O<sub>5</sub> heterojunctions. This approach will propel the further development of nano-lithography techniques for functional device applications of 2D materials.