Broadband near-infrared hyperbolic polaritons in MoOCl<sub>2</sub>.
basic_science · Level V
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- Record sourced from PubMed, PMID 40615505.
- Also identified by DOI 10.1038/s41467-025-61548-w and PMC identifier 12227530.
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Abstract
Hyperbolic polaritons have drawn great attention in nanoscale light manipulation due to their unique properties. Currently, most studies focus on natural hyperbolic phonon materials in the mid-infrared, limiting their application in the visible to near-infrared range. Here, we present a work on broadband near-infrared hyperbolic plasmon polaritons in a van der Waals material MoOCl<sub>2</sub> by a perturbation-free direct imaging technique of photoemission electron microscopy. In particular, the hyperbolic polariton behavior has been dynamically tailored and manipulated by wavelength, polarization, interlayer twist, and artificial structure, providing a reconfigurable platform for nanophotonic applications. Notably, the full iso-frequency contours can be reconstructed via polarization-selective excitations. Our work has contributed to hyperbolic materials in the broadband near-infrared with MoOCl<sub>2</sub>, and has revealed PEEM to be an ideal method for studying hyperbolic plasmon polaritons at the space-time limit.