Coherent spectroscopy with a single antiproton spin.

Latacz, B M; Erlewein, S R; Fleck, M; Jäger, J I; Abbass, F; Arndt, B P; Geissler, P; Imamura, T et al. · Nature · 2025

basic_science · Level V

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Abstract

Coherent quantum transition spectroscopy is a powerful tool in metrology<sup>1</sup>, quantum information processing<sup>2</sup>, magnetometry<sup>3</sup> and precision tests of the standard model<sup>4</sup>. It was applied with great success in proton and deuteron magnetic moment measurements<sup>5</sup>, which culminated in maser spectroscopy with sub-parts-per-trillion resolution<sup>6</sup> and many other experiments at the forefront of physics<sup>7</sup>. All of these experiments were performed on macroscopic ensembles of particles, whereas the coherent spectroscopy of a 'free' single nuclear spin has, to our knowledge, never been reported before. Here we demonstrate coherent quantum transition spectroscopy of the spin of a single antiproton stored in a cryogenic Penning-trap system. We apply a multi-trap technique<sup>8</sup>, detect the antiproton spin state using the continuous Stern-Gerlach effect<sup>9</sup> and transport the particle to the homogeneous magnetic field of a precision trap (PT). Here we induce the coherent dynamics and analyse the result by quantum-projection measurements in the analysis trap (AT)<sup>10</sup>. We observe, for the first time, Rabi oscillations of an antiproton spin and achieve in time-series measurements spin-inversion probabilities greater than 80% at spin coherence times of about 50 s. Scans of single-particle spin resonances show inversions greater than 70%, at transition linewidths 16 times narrower than in previous measurements<sup>8</sup>, limited by cyclotron frequency measurement decoherence. This achievement marks a notable step towards at least tenfold improved tests of matter/antimatter symmetry using proton and antiproton magnetic moments.