Fine-structure constant sensitivity of the Th-229 nuclear clock transition.

Beeks, Kjeld; Kazakov, Georgy A; Schaden, Fabian; Morawetz, Ira; Toscani De Col, Luca; Riebner, Thomas; Bartokos, Michael; Sikorsky, Tomas et al. · Nat Commun · 2025

basic_science · Level V

Where this comes from

Abstract

Nuclear laser spectroscopy at the 10<sup>-12</sup> precision level (Nature 633.8028 (2024): 63-70) determined the fractional change in the nuclear quadrupole moment of <sup>229</sup>Th upon excitation, ΔQ<sub>0</sub>/Q<sub>0</sub> = 1.791(2)%. Such high-accuracy nuclear parameters enable stringent tests and refinement of <sup>229</sup>Th nuclear models. Using a semi-classical prolate-spheroid model, we quantify the transition frequency's sensitivity to fine-structure constant variations as K = 5900(2300), with uncertainty dominated by the measured charge-radius change Δ〈r<sup>2</sup>〉. This supports the predicted higher α-sensitivity of nuclear clocks over atomic clocks, important for new-physics searches. We find ΔQ<sub>0</sub> strongly dependent on nuclear volume, challenging the constant-volume approximation. The deviation between measured and predicted ΔQ<sub>0</sub>/Q<sub>0</sub> underlines the need for improved modeling and measurement of additional nuclear parameters. We explicitly assess the octupole contribution to α-sensitivity.