Structural insights into AQP3 channel closure upon pH and redox changes reveal an autoregulatory molecular mechanism.

Huang, Peng; Venskutonytė, Raminta; Wilson, Carter J; Bsharat, Sara; Prasad, Rashmi B; Gourdon, Pontus; Artner, Isabella; de Groot, Bert L et al. · Nat Commun · 2025

basic_science · Level V

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Abstract

Regulation of intracellular levels of reactive oxygen species (ROS) remains poorly understood. Aquaporin 3 (AQP3) facilitates the membrane transport of hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>), a key ROS signaling molecule. Here we elucidate the molecular mechanism of AQP3 and show that its regulatory properties are both pH dependent and autoregulated by H<sub>2</sub>O<sub>2</sub>. Using single particle cryo-electron microscopy, we present open and closed conformations of human AQP3. At pH 8.0, the channel adopts an open state, while acidic pH or exposure to H<sub>2</sub>O<sub>2</sub> promotes closure via a large conformational rearrangement of extracellular loop E. These findings reveal a mechanism for autoregulation of H<sub>2</sub>O<sub>2</sub> transport and establish AQP3 as a key modulator of redox homeostasis in human pancreatic β-cells.

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