Exciton-Defect Interaction and Optical Properties from a First-Principles T-Matrix Approach.

Chan, Yang-Hao; Haber, Jonah B; Naik, Mit H; Qiu, Diana Y; da Jornada, Felipe H · Nano Lett · 2026

basic_science · Level V

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Abstract

Understanding exciton-defect interactions is critical for optimizing optoelectronic and quantum information applications in many materials. However, <i>ab initio</i> simulations of material properties with defects are often limited to high defect density. Here, we study effects of exciton-defect interactions on optical absorption and photoluminescence spectra in monolayer MoS<sub>2</sub> using a first-principles T-matrix approach. We demonstrate that exciton-defect bound states can be captured by the disorder-averaged Green's function with the T-matrix approximation and further analyze their optical properties. Our approach yields photoluminescence spectra in good agreement with experiments and provides a new, computationally efficient framework for simulating optical properties of disordered 2D materials from first-principles.