Enhancement of the Unconventional Spin-Orbit Torque Efficiency through Kagome Orientation Engineering in Epitaxial Noncollinear Antiferromagnet Mn<sub>3</sub>Sn.
basic_science · Level V
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- Record sourced from PubMed, PMID 41546642.
- Also identified by DOI 10.1021/acs.nanolett.5c04920.
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Abstract
Noncollinear antiferromagnets show great potential for next-generation spintronic devices due to their unique spin textures and ultrafast dynamics, with Kagome-lattice Mn<sub>3</sub>Sn a key spin-orbit torque (SOT) candidate enabled by room-temperature unconventional spin polarization. However, the impact of crystal orientation on its SOT efficiency remains unaddressed. Herein, we combine experiments and first-principles calculations to investigate Kagome-facet-dependent unconventional out-of-plane SOT in Mn<sub>3</sub>Sn, confirming <i>z</i>-direction polarized spin current and unconventional spin polarization in the material. Strikingly, (112̅0)-oriented Mn<sub>3</sub>Sn films exhibit 13-fold higher unconventional SOT efficiency ξ<sub><i>z</i></sub> associated with <i>z</i>-direction spin polarization than (0002)-oriented counterparts, a behavior governed by Kagome lattice symmetry and facet-dependent spin transport. First-principles calculations further verify the Kagome plane's critical role in enhancing anisotropic spin textures and transport properties. This crystal-facet engineering strategy resolves the longstanding ambiguity in SOT anisotropy of noncollinear antiferromagnets and establishes Mn<sub>3</sub>Sn as a versatile platform for energy-efficient antiferromagnetic spintronic devices.