Absence of Transport Altermagnetic Spin-Splitting Effect in RuO<sub>2</sub>.

Wang, Yu-Chun; Shen, Zhe-Yu; Lin, Chia-Hsi; Hsu, Wei-Chih; Chen, You-Sheng; Chin, Yi-Ying; Singh, Akhilesh Kr; Lee, Wei-Li et al. · Nano Lett · 2026

basic_science · Level V

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Abstract

Altermagnets have attracted significant interest recently. Through the altermagnetic spin-splitting effect (ASSE), a longitudinal spin-polarized or a transverse pure spin current can be generated upon charge current injection. The ASSE is a key experimental feature for altermagnets but is often mixed with the spin Hall effect (SHE). Here, we present a comprehensive study of spin-to-charge conversion in epitaxial ruthenium dioxide (RuO<sub>2</sub>) thin films using the ferromagnetic insulator yttrium iron garnet (YIG) as the spin current source. We conclusively show the absence of the ASSE in RuO<sub>2</sub> films grown with three different crystal orientations. Instead, we attribute the spin-to-charge conversion signals solely to the SHE. Moreover, we reveal a negative spin Hall angle in RuO<sub>2</sub> when it is adjacent to YIG, which reverses the sign when interfaced with Py. Our study provides crucial insights into the recent arguments on RuO<sub>2</sub> and advances the understanding of spin-to-charge conversion in low-symmetry materials.