Van der Waals Ferroelectric CuInP<sub>2</sub>S<sub>6</sub>-based Multi-slope In-memory Probabilistic Computing.

Kim, Changyoung; Kim, Namju; Kang, Seongkweon; Park, Chang Yong; Lee, Sang-Min; Jang, Cheolhwa; Park, Ji-Sang; Jang, Byung Chul et al. · Adv Mater · 2026

basic_science · Level V

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Abstract

Probabilistic bit (p-bit) is the fundamental building block and core element of probabilistic computing (p-computing). However, physical separation of bit generation and memory storage creates a memory bottleneck in conventional p-computing architectures. We report on experimentally integrating voltage-tunable stochastic bit generation and non-volatile memory functionalities within a single in-memory device to realize a p-bit with van der Waals ferroelectric CuInP<sub>2</sub>S<sub>6</sub> (CIPS). Leveraging the stochastic displacement of Cu<sup>+</sup> ions and the material's remanent polarization under an external electric field, the proposed device achieves stable random bit retention (>1000 s) with low power consumption (∼75 nW). This eliminates the need for data transfer between separate memory and logic units, thereby enabling efficient in-memory p-computing with improved system-level performance. In-memory p-computing outperforms conventional p-computing in device-to-system-level NP-hard simulations, reducing time-complexity from O(n<sup>2</sup>) to O(n<sup>1.5</sup>). Notably, the sigmoid slope of the probabilistic output is dynamically tuned by varying the CIPS layer thickness, enabling adaptive control over exploration-exploitation characteristics. Broader slopes facilitate initial exploration, whereas steeper slopes support rapid convergence in later stages. Sigmoid slope tunability over a wide dynamic range (6.17-38.41) reduces convergence steps by 400-fold, highlighting the potential of CIPS-based p-bit as a compact, energy-efficient platform for scalable and adaptive p-computing.