Topological metal-insulator transition within the ferromagnetic state.

Forslund, Ola Kenji; Ong, Chin Shen; Hirschmann, Moritz M; Gauthier, Nicolas; Uchiyama, Hiroshi; Tzschaschel, Christian; Mazzone, Daniel G; Sibille, Romain et al. · Nat Commun · 2026

basic_science · Level V

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Abstract

A major challenge in condensed matter physics is integrating topological phenomena with correlated electron physics to leverage both types of states for next-generation quantum devices. Metal-insulator transitions are central to bridging these two domains while simultaneously serving as on-off switches for electronic states. Here, we demonstrate how the prototypical material of K<sub>2</sub>Cr<sub>8</sub>O<sub>16</sub> undergoes a ferromagnetic metal-insulator transition accompanied by a change in band topology. Through inelastic x-ray and neutron scattering experiments combined with first-principles theoretical calculations, we show that this transition is not driven by a Peierls mechanism, given the lack of phonon softening. Instead, we establish the transition as a topological metal-insulator transition within the ferromagnetic phase with potential axionic properties, where electron correlations play a key role in stabilizing the insulating state. These results reveal how a metal-insulator transition provides a pathway through which magnetism, topology, and electronic correlations interact.