Probing ultrafast heating and ionization dynamics in solid density plasmas with time-resolved resonant X-ray absorption and emission.

Huang, Lingen; Mishchenko, Mikhail; Šmíd, Michal; Humphries, Oliver S; Preston, Thomas R; Pan, Xiayun; Yang, Long; Hagemann, Johannes et al. · Nat Commun · 2026

basic_science · Level V

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Abstract

Heating and ionization are among the most fundamental processes in relativistic laser-solid interactions; however, their spatiotemporal evolution remains challenging to capture experimentally. Here we present detailed diagnosis of high-intensity laser interactions with wire targets, leveraging the extreme spectral brightness of an X-ray free-electron laser in sub-picosecond time-resolved resonant X-ray emission spectroscopy and absorption imaging. Experimental results are compared with comprehensive simulations using atomic collisional-radiative models, particle-in-cell, and magnetohydrodynamics codes to elucidate the underlying physics. These multi-scale simulations reveal extreme sensitivity of basic plasma parameters with widely used models, such as temperature and ionization depth, which are able to be constrained by incorporating a detailed accounting of laser spatial profiles, pre-plasma conditions, and collisional processes. These results provide new insights into heating and ionization dynamics in the high-energy-density regime relevant to inertial fusion energy research, both as an experimental platform for accessing theoretically challenging conditions and as a benchmark for improving models of high-power laser-plasma interactions.