Carbon Nanotube-Aramid Fiber Enabled Dielectric Dispersion in Paper Composites for Ultrabroadband Lightweight Absorbers.

Liu, Sicheng; Huang, Zhengsheng; Tian, Huahui; Cheng, Yao; Hao, He; Xia, Chenbin; Long, Jin; Hu, Jian et al. · Nano Lett · 2026

basic_science · Level V

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Abstract

Lightweight broadband microwave-absorbing materials (MAMs) are important for stealth and electromagnetic protection, but conventional designs usually rely on thick structures or high-load magnetic fillers, which often impose substantial weight penalties. Here, we introduce a dielectric-dispersion engineering strategy in aramid paper composites, enabled by single-walled carbon nanotube-coated aramid fibers (SAFs). In this system, both fiber length and conductivity are tunable, enabling regulation of the frequency-dependent permittivity through anisotropic depolarization effects. Multiscale simulations and experiments identify dielectric dispersion regulation as the key mechanism governing broadband absorption. SAFs with a length of 18 mm (about 1.28 × 10<sup>4</sup> S/m) enable broadband absorption spanning 2.2-18 GHz, whereas 9 mm SAFs deliver enhanced performance in the S-band (2.0-4.0 GHz). Guided by this principle, a gradient Jaumann absorber (18.5 mm, 40 kg/m<sup>3</sup>) achieves full-band absorption across 2.0-18 GHz. This work offers a conductive-fiber platform and insights for lightweight, high-performance MAMs.