Direct observation of the superallowed α-decay of ¹⁰⁴Te.

Abstract

The radioactivity of the α particle is among the most compelling evidence for the existence of cluster structures in atomic nuclei. During the decay process, a pre-existing α particle tunnels through the potential barrier formed by the residual nucleus^1,2. The degree of preformation of the α particle, a strongly bound system of two protons and two neutrons, is extracted from the data by dividing the α-decay probability by the barrier penetrability for a given particle energy. The preformation probability changes rapidly near nuclear shell closures, which is direct evidence that clustering is connected to nuclear structure³. Enhanced preformation was observed in the lightest α-particle emitters, spherical tellurium and xenon isotopes decaying to magic isotopes of tin. Here we show the most extreme case of α-particle preformation from the measurement of the decay of tellurium-104 (¹⁰⁴Te). With a half-life of <math xmlns="http://www.w3.org/1998/Math/MathML"><mn>7.</mn> <msubsup><mrow><mn>2</mn></mrow> <mrow><mo>-</mo> <mn>1.5</mn></mrow> <mrow><mo>+</mo> <mn>2.3</mn></mrow> </msubsup> <mspace></mspace> <mrow><mrow><mi>ns</mi></mrow> </mrow> </math> , ¹⁰⁴Te is the fastest ground-state α-emitting nucleus known so far. The deduced preformation demonstrates that the enhancement is greater for ¹⁰⁴Te than for any other nucleus. One nuclear model that can explain our observation postulates that the α particle can exist only in the low-nuclear-matter-density regions on the surface of the nucleus. The uniquely high preformation for ¹⁰⁴Te is attributed to its relation to doubly magic tin-100 (¹⁰⁰Sn), creating conditions conducive to form an α particle.